Download e-book for kindle: Asymmetric catalysis in organic synthesis by Ryoji Noyori

By Ryoji Noyori

Offers with uncomplicated ideas of uneven catalysis concentrating on its artificial value. Covers homogeneous uneven hydrogenation, uneven catalysis through chiral steel complexes, heterogeneous catalysis and non-organometallic catalysis. the gathering of more than a few stereoselective reactions illustrate a number of options and methodologies in addition to their normal application.

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Extra resources for Asymmetric catalysis in organic synthesis

Sample text

Of l and 7 t-ButYl hydroperoxide osiR3 /* I I l I o2'\r" l - l "'l;3il'i" il. coocH3 48"/. -coocH, (Bzt)zN, /z-CO PrcH) 1 (E)-2 AcOH, H2O 51o/" coocH3 4 retro-aldolreaction' can be convertedinto 4 by a equiv. ii,'="*"o,"". ''( H 1,NEt3 --sr%- \ \- / ' \ " H I I cn"orc-'\r? R3sio /l *-) il ll4' and K' Fukumoto'Am' Soc'' I M. Ihara,M. Ohnishi,M' Takano'K' Makita'N' Taniguchi' 4408 (1ee2). i M . T . R e e t za n d E . r*rn y-dibenzvlaminoof chiraty-aminoenoates. Since since (16, 30a) and reduced with high stereoselectivity can be 'iii-""0**" Reetzr has B_keto esters stereoselective"up'uit addition' r-BuooH with 7-dibenzylaminoenoates epoxidation substrates(1).

E. Mark

In contrast,basic elimination and protiodesilylationprovides sarohorneneC (7) with high selectivity. :hlC. (cH3)3si r ' I l()91). ACHz 1) KH ,0" (99%) 2) F (68%) 7 : T. Matsumoto, M Kat-sut Scheme r r2R)-2-r-ButYl-6mahf An imProved PrePan e r R)-3-hYdroxYbutanotc I scale I large a acid on 48' 4087(1992)' Nakai'Tetrahedron' rN. Kishi,T. Maeda,K' Mikami' andT' c(cH3)3 "*t:#::#-,:;ffi:l-J,:J::;tll''o'^o^^'ion suchas derivative or ananthracene or C11; occurs mainly at Ce a problem sin-e attack o;;-;;t' alkyllithium t-BuOlJBuLi an with with 1 "un O" cffected ;; ;'' o'tho-M"tuluti"n give the instead of desired utt"tk with (CHr)lrSnCl to '"u"tion Uy at 190" follo*td treatment on (5 equiv.

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Asymmetric catalysis in organic synthesis by Ryoji Noyori


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